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I don't buy slabbed coins so I pass on all of them.
This.
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Personally wouldn't buy either of the choices, not into having to have the high grades
And this.
(Also either of those coins is likely to be far too expensive for my collection, which is yet
another reason for me to avoid them, but let's ignore that for the moment. Maybe I just got a remote job for a US company and now earn $10+ per hour.)
Assuming that I do, in fact, need one (for example, if this particular date or type is rare in circulated grade
and has counterfeiting problems that mean non-slabbed coins are suspect[1]), I'm probably going to agree with Jbuck's reasoning and take the 66 - I could hardly care less about CAC; of course I don't care much about PCGS either, but if I do end up with a MS grade slab I'd rather take the higher number.
[1] limiting this to coins that are common in grades as low as MS-65 (which excludes, for example, Platinum Eagles), the first thing that comes to mind is some kind of classic commemorative, but there are probably other options I couldn't think of immediately